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NO_x and H₂S formation in the reductive zone of air-staged combustion of

Jinzhi CAI, Dan LI, Denggao CHEN, Zhenshan LI

《能源前沿（英文）》 2021年第15卷第1期页码 4-13 doi: 10.1007/s11708-020-0804-y

摘要： Low NO combustion of blended coals is widely used in coal-fired boilers in China to control NO emission; thus, it is necessary to understand the formation mechanism of NO and H S during the combustion of blended coals. This paper focused on the investigation of reductive gases in the formation of NO and H S in the reductive zone of blended coals during combustion. Experiments with Zhundong (ZD) and Commercial (GE) coal and their blends with different mixing ratios were conducted in a drop tube furnace at 1200°C–1400°C with an excessive air ratio of 0.6–1.2. The coal conversion and formation characteristics of CO, H S, and NO in the fuel-rich zone were carefully studied under different experimental conditions for different blend ratios. Blending ZD into GE was found to increase not only the coal conversion but also the concentrations of CO and H S as NO reduction accelerated. Both the CO and H S concentrations inblended coal combustion increase with an increase in the combustion temperature and a decrease in the excessive air ratio. Based on accumulated experimental data, one interesting finding was that NO and H S from blended coal combustion were almost directly dependent on the CO concentration, and the CO concentration of the blended coal combustion depended on the single char gasification conversion.Thus, CO, NO , and H S formation characteristics from blended coal combustion can be well predicted by single char gasification kinetics.

关键词： blended coal combustion NO_xformation H₂S formation air staged combustion

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Effect of Fe on NO release during char combustion in air and O

Ying GU, Xiaowei LIU, Bo ZHAO, Minghou XU

《能源前沿（英文）》 2012年第6卷第2期页码 200-206 doi: 10.1007/s11708-012-0181-2

摘要： The chemistry of char was probed by studying nitrogen release under the reactions with air and oxy-fuel combustion. The experiments were conducted in a drop tube furnace and a fixed bed flow reactor. NO was observed during those experiments. The results show that the particle size of char generated at 1073 K in CO is larger than that in N . However, at 1573 K, it is smaller in CO atmosphere due to particle breaking by gasification of char and CO . The Fe addition increases the NO conversion ratio, and the effect of Fe rises steeply with the process going until it becomes stable in the end. The results also indicate that the release of NO increases more significantly with the Fe addition in oxy-fuel environment.

关键词： NO Fe char combustion CO₂

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Experimental study of humid air reverse diffusion combustion in a turbulent flow field

GE Bing, ZANG Shusheng, GU Xin

《能源前沿（英文）》 2007年第1卷第4期页码 428-434 doi: 10.1007/s11708-007-0062-6

摘要： Experiments were performed to investigate the differences between the propane/air turbulent diffusion reactive flows past bluff-body and the propane/humid air turbulent diffusion reactive flows in the same conditions. The velocity

关键词： propane/humid propane/air turbulent bluff-body turbulent diffusion

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Experimental study on premixed combustion of spherically propagating methanol-air-nitrogen flames

Xiangang WANG, Zhiyuan ZHANG, Zuohua HUANG, Xibin WANG, Haiyan MIAO,

《能源前沿（英文）》 2010年第4卷第2期页码 223-233 doi: 10.1007/s11708-010-0016-y

摘要： The outward propagation and development of surface instability of the spark-ignited spherical premixed flames for methanol-air-nitrogen mixtures were experimentally studied by using a constant volume combustion chamber and a high-speed schlieren photography system. The laminar burning velocities, the mass burning fluxes, and the Markstein lengths were obtained at different equivalence ratios, dilution ratios, initial temperatures, and pressures. The laminar burning velocities and the mass burning fluxes give a similar curve versus the equivalence ratios. They increase with the increase of initial temperature and decrease with the increase of dilution ratio. The laminar burning velocity decreases with elevating the initial pressure, while the mass burning flux increases with the increase of the initial pressure. Markstein length decreases slightly with the increase of initial temperature for the rich mixtures. High initial pressure corresponds to low Markstein length. Markstein length increases with the increase of dilution ratio, which is more obvious when the mixture becomes leaner. Equivalence ratio has a slight impact on the development of the diffusive-thermal cellular structure at elevated initial pressures. The initial pressure has a significant influence on the occurrence of the flame front cellular structure. At the elevated pressures, the cracks on the flame surface branch and develop into the cell structure. These cells are bounded by cracks emitting a bright light, which may indicate soot formation. For very lean mixture combustion, the buoyancy effect and cooling effect from the spark electrodes have a significant impact on the flame propagation. The hydrodynamic instability, inhibited with the increase of initial temperature around the stoichiometric equivalence ratio, is enhanced with the increase of initial pressure and suppressed by mixture dilution.

关键词： methanol spherical flame propagation characteristics flame instabilities

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Modeling and simulation analysis on parallel hybrid air-fuel vehicle

Pinglu CHEN, Xiaoli YU, Xianghong NIE, Yidong FANG

《能源前沿（英文）》 2010年第4卷第4期页码 553-559 doi: 10.1007/s11708-010-0008-y

摘要： Based on the vehicle simulation software ADVISOR, the model of a parallel air-fuel hybrid vehicle was established, and the modeling of an air powered engine (APE), heat exchanger, braking air tank and control strategy were discussed in detail. Using the vehicle model, a hybrid vehicle refitted from a traditional diesel car was analyzed. The results show that for the New European Driving Cycle (NEDC), the Urban Dynamometer Driving Schedule (UDDS) and the Highway Fuel Economy Test (HWFET) driving cycle, the total reductions in fossil fuel consumption of the hybrid vehicle were 48.29%, 48.51% and 22.07%, respectively, and the emissions could be decreased greatly compared with the traditional diesel car, while the compressed air consumptions of the hybrid vehicle were 97.366, 85.292 and 56.358 kg/100 km, respectively. Using the diesel equivalent as the indicator of fuel economy, the hybrid vehicle could improve the fuel economy by 14.71% and 16.75% for the NEDC and the UDDS driving cycles and decrease by 5.04% for the HWFET driving cycle compared with the traditional car. The simulation model and analysis in this paper could act as the theoretical basis and research platform in optimizing the key components and control strategy of hybrid air-fuel vehicles.

关键词： air powered engine hybrid vehicle internal combustion engine simulation

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Numerical simulation of bituminous coal combustion in a full-scale tiny-oil ignition burner: influenceof excess air ratio

Zhengqi LI, Chunlong LIU, Xiang ZHANG, Lingyan ZENG, Zhichao CHEN

《能源前沿（英文）》 2012年第6卷第3期页码 296-303 doi: 10.1007/s11708-012-0191-0

摘要： The progression of ignition was numerically simulated with the aim of realizing a full-scale tiny-oil ignition burner that is identical to the burner used in an 800 MWe utility boiler. The numerical simulations were conducted for four excess air ratios, 0.56, 0.75, 0.98 and 1.14 (corresponding to primary air velocities of 17, 23, 30 and 35 m/s, respectively), which were chosen because they had been used previously in practical experiments. The numerical simulations agreed well with the experimental results, which demonstrate the suitability of the model used in the calculations. The gas temperatures were high along the center line of the burner for the four excess air ratios. The flame spread to the burner wall and the high-temperature region was enlarged in the radial direction along the primary air flow direction. The O concentrations for the four excess air ratios were 0.5%, 1.1%, 0.9% and 3.0% at the exit of the second combustion chamber. The CO peak concentration was very high with values of 7.9%, 9.9%, 11.3% and 10.6% for the four excess air ratios at the exit of the second combustion chamber.

关键词： numerical simulation tiny-oil ignition burner pulverized coal temperature field

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Industrial-scale investigations on effects of tertiary-air declination angle on combustion and steam

Xiaoguang LI, Lingyan ZENG, Hongye LIU, Yao LI, Yifu LI, Yunlong ZHAO, Bo JIAO, Minhang SONG, Shaofeng ZHANG, Zhichao CHEN, Zhengqi LI

《能源前沿（英文）》 2021年第15卷第1期页码 132-142 doi: 10.1007/s11708-020-0803-z

摘要： Industrial-scale experiments were conducted to study the effects of tertiary air declination angle (TDA) on the coal combustion and steam temperature characteristics in the first 350-MW supercritical down-fired boiler in China with the multiple-injection and multiple-staging combustion (MIMSC) technology at medium and high loads. The experimental results indicated that as the TDA increased from 0° to 15°, the overall gas temperature in the lower furnace rose and the symmetry of temperature field was enhanced. The ignition distance of the fuel-rich coal/air flow decreased. In near-burner region, the concentration of O decreased while the concentrations of CO and NO increased. The concentration of NO decreased in near-tertiary-air region. The carbon in fly ash decreased significantly from 8.40% to 6.45% at a load of 260 MW. At a TDA of 15°, the ignition distances were the shortest (2.07 m and 1.73 m) at a load of 210 MW and 260 MW, respectively. The main and reheat steam temperatures were the highest (557.2°C and 559.4°C at a load of 210 MW, 558.4°C and 560.3°C at a load of 260 MW). The carbon in fly ash was the lowest (4.83%) at a load of 210 MW. On changing the TDA from 15° to 25°, the flame kernel was found to move downward and the main and reheat steam temperatures dropped obviously. The change of TDA has little effect on NO emissions(660–681 mg/m at 6% O ). In comprehensive consideration of the pulverized coal combustion characteristics and the unit economic performance, an optimal TDA of 15° is recommended.

关键词： supercritical down-fired boiler industrial-scale experiment tertiary air declination angle coal combustion steam temperature

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基于煤炭分级转化的发电技术前景

岑可法,倪明江,骆仲泱,方梦祥,王勤辉,王智化,岑建孟

《中国工程科学》 2015年第17卷第9期页码 118-122

摘要：

面对我国一次能源以煤为主、能源需求日益增长以及大气环境持续恶化的现实，构建资源、能源、环境一体化的可持续发展能源系统是我国能源的战略方向。本文介绍了基于“煤炭既是能源又是资源”的理念提出的煤炭转化利用新技术——煤炭分级转化发电技术的路线和特点。从节能减排等方面对该技术的发展前景进行了展望，指出煤炭分级转化的发电技术可提高煤炭发电的综合效益，改变煤炭单一用于发电的产业结构，可形成基于煤炭资源化利用发电的新产业链并缓解我国油气等资源的紧缺状况，对于改变和优化国家煤电产业结构、循环经济和节能减排具有重要意义。

关键词：分级转化；梯级利用；节能减排；煤炭

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A logic-based controller for the mitigation of ventilation air methane in a catalytic flow reversal reactor

Zhikai LI, Zhangfeng QIN, Yagang ZHANG, Zhiwei WU, Hui WANG, Shuna LI, Mei DONG, Weibin FAN, Jianguo WANG

《化学科学与工程前沿（英文）》 2013年第7卷第3期页码 347-356 doi: 10.1007/s11705-013-1347-0

摘要： The control system of a catalytic flow reversal reactor (CFRR) for the mitigation of ventilation air methane was investigated. A one-dimensional heterogeneous model with a logic-based controller was applied to simulate the CFRR. The simulation results indicated that the controller developed in this work performs well under normal conditions. Air dilution and auxiliary methane injection are effective to avoid the catalyst overheating and reaction extinction caused by prolonged rich and lean feed conditions, respectively. In contrast, the reactor is prone to lose control by adjusting the switching time solely. Air dilution exhibits the effects of two contradictory aspects on the operation of CFRR, i.e., cooling the bed and accumulating heat, though the former is in general more prominent. Lowering the reference temperature for flow reversal can decrease the bed temperature and benefit stable operation under rich methane feed condition.

关键词： ventilation air methane reverse flow reactor lean methane combustion logic-based controller mathematical modeling

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Thermogravimetric kinetic analysis of

SUKARNI,SUDJITO,Nurkholis HAMIDI,Uun YANUHAR,I.N.G. WARDANA

《能源前沿（英文）》 2015年第9卷第2期页码 125-133 doi: 10.1007/s11708-015-0346-x

摘要： The thermal behavior of combustion in air atmosphere were investigated by performing experiments on STA PT1600 Thermal Analyzer at heating rates of 10°C/min, 40°C/min and 70°C/min and range of temperatures from room temperature to 1200°C. The kinetic parameters were evaluated by using Kissinger and Ozawa methods. The result showed that combustion occurred in five stages. Started with initial devolatilization, the main thermal decomposition and combustion process, transition stage, the combustion of char and the last stage was the slow burning reaction of residual char. In line with increasing heating rate, the mass loss rate increased as well, but it delayed the thermal decomposition processes toward higher temperatures. The average activation energy at the main thermal decomposition stage and the stage of char combustion were approximately 251 kJ/mol and 178 kJ/mol, respectively.

关键词： Nannochloropsis oculata combustion kinetic parameters air atmosphere thermogravimetric

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风包粉系列浓淡煤粉燃烧技术的研究

秦裕琨,李争起,孙锐,陈力哲,孙绍增,朱群益,李瑞扬,高继慧,吴少华

《中国工程科学》 2002年第4卷第11期页码 42-49

摘要：

总结了哈尔滨工业大学15年来对浓淡煤粉燃烧技术的研究成果，阐述了浓淡煤粉燃烧技术的原理及所具有的风包粉流动特点，并通过工业试验验证了风包粉原理。针对我国电站锅炉燃煤的特点，提出了需要解决的5个问题，指出了浓淡燃烧技术的发展方向。

关键词：锅炉燃烧器浓淡燃烧 NO_x

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A Review on Shale Gas Development in Fuling

Zhi-gang Wang

《工程管理前沿（英文）》 2015年第2卷第1期页码 76-81 doi: 10.15302/J-FEM-2015011

摘要： The Fuling Marine Shale Deposit contains vast gas resources. Due to tectonic activities, complex surface and geological conditions, significant differences make it unlike that of North America. Thus, it is not suitable to completely copy the technology and the development model from North America. Therefore we need engineering technology and a business development model fit for Fuling Shale Gas Development (FSGD). Through difficulties and characteristics analysis of the shale gas development area, we determined geological engineering design methods and integrated workflow, established a series of the core technologies, including horizontal well drilling with long laterals, staged fracturing and completion technology, developed main fluids, tools and equipment, put forward “well factory” mode in mountain region and “full cycle learning and system optimization” management methods. Break through was made in China’s first large-scale shale gas fields commercial development. By the end of 2014, production capacity reached 25 × 10 m /a, and cumulative gas production reached 12.24 × 10 m , which made a solid foundation to build production capacity of 50 × 10 m /a in 2015 and 100 × 10 m /a in 2017. Not only has FSGD established a demonstration for the other shale gas fields’ development, but also will be taken as reference to other large and extra-large construction projects of the industry.

关键词： Fuling shale gas drilling and completion staged fracturing learning curve capacity building commercial development

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Combustion characteristics and kinetics of bio-oil

Ruixia ZHANG, Zhaoping ZHONG, Yaji HUANG

《化学科学与工程前沿（英文）》 2009年第3卷第2期页码 119-124 doi: 10.1007/s11705-009-0068-x

摘要： The combustion characteristics of bio-oils derived from rice husk and corn were studied by thermogravimetry analysis. According to the thermogravimetry (TG), differential thermogravimetry (DTG) and differential thermal analysis (DTA) curves of bio-oils in air and nitrogen atmosphere, we analyzed the combustion characteristics of different kinds of bio-oils in different atmospheres and worked out the combustion kinetics parameters of the bio-oil, providing reliable base data for the burning of bio-oil. The thermogravimetry indicated that the combustion process of bio-oil was divided into three stages. At the same time, the combustion process can be described by different order reaction models, and with the method of Coats-Redfern, the activation energy and frequency factor of different kinds of bio-oils were obtained.

关键词： bio-oil combustion characteristics combustion kinetics

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Numerical simulation of laminar premixed combustion in a porous burner

ZHAO Pinghui, CHEN Yiliang, LIU Minghou, DING Min, ZHANG Genxuan

《能源前沿（英文）》 2007年第1卷第2期页码 233-238 doi: 10.1007/s11708-007-0032-8

摘要： Premixed combustion in porous media differs substantially from combustion in free space. The interphase heat transfer between a gas mixture and a porous medium becomes dominant in the premixed combustion process. In this paper, the premixed combustion of CH

关键词： interphase mixture dominant Premixed combustion premixed combustion

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Entropy production analysis of swirling diffusion combustion processes

Deodat MAKHANLALL, Linhua LIU,

《能源前沿（英文）》 2010年第4卷第3期页码 326-332 doi: 10.1007/s11708-009-0058-1

摘要： A critical factor in the design of combustion systems for optimum fuel economy and emission performance lies in adequately predicting thermodynamic irreversibilities associated with transport and chemical processes. The objective of this study is to map these irreversibilities in terms of entropy production for methane combustion. The numerical solution of the combustion process is conducted with the help of a Fluent 6.1.22 computer code, and the volumetric entropy production rate due to chemical reaction, viscous dissipation, and mass and heat transfer are calculated as post-processed quantities with the computed data of the reaction rates, fluid velocity, temperature and radiative intensity. This paper shows that radiative heat transfer, which is an important source of entropy production, cannot be omitted for combustion systems. The study is extended by conducting a parametric investigation to include the effects of wall emissivity, optical thickness, swirl number, and Boltzmann number on entropy production. Global entropy production rates decrease with the increase in swirl velocity, wall emissivity and optical thickness. Introducing swirling air into the combustion system and operations with the appropriate Boltzmann number reduces the irreversibility affected regions and improves energy utilization efficiency.

关键词： entropy-based design radiation transfer swirl magnussen combustion-model